Nanomaterials (Dec 2022)

Critical Effect of Oxygen Pressure in Pulsed Laser Deposition for Room Temperature and High Performance Amorphous In-Ga-Zn-O Thin Film Transistors

  • Yue Zhou,
  • Dao Wang,
  • Yushan Li,
  • Lixin Jing,
  • Shuangjie Li,
  • Xiaodan Chen,
  • Beijing Zhang,
  • Wentao Shuai,
  • Ruiqiang Tao,
  • Xubing Lu,
  • Junming Liu

DOI
https://doi.org/10.3390/nano12244358
Journal volume & issue
Vol. 12, no. 24
p. 4358

Abstract

Read online

The aspects of low processing temperature and easy running in oxygen atmosphere contribute to the potential of pulsed laser deposition (PLD) in developing a-IGZO TFTs for flexible applications. However, the realization of low-temperature and high-performance devices with determined strategies requires further exploration. In this work, the effect of oxygen pressure and post-annealing processes and their mechanisms on the performance evolution of a-IGZO TFTs by PLD were systematically studied. A room-temperature a-IGZO TFT with no hysteresis and excellent performances, including a μ of 17.19 cm2/V·s, an Ion/Ioff of 1.7 × 106, and a SS of 403.23 mV/decade, was prepared at the oxygen pressure of 0.5 Pa. Moreover, an O2 annealing atmosphere was confirmed effective for high-quality a-IGZO films deposited at high oxygen pressure (10 Pa), which demonstrates the critical effect of oxygen vacancies, rather than weak bonds, on the device’s performance.

Keywords